基于脉冲整形的激发双重态间的相干布局操控

王贞浩; 张杨华; 王全军; 丁晶洁; 刘作业

doi:10.7510/jgjs.issn.1001-3806.2016.06.002

基于脉冲整形的激发双重态间的相干布局操控

1.
兰州大学核科学与技术学院, 兰州 730000

作者简介: 王贞浩(1994-),男,硕士研究生,现主要从事基于飞秒脉冲的瞬态吸收谱测量的研究。.

通讯作者: 刘作业, zyl@lzu.edu.cn

基金项目:
国家自然科学基金资助项目（11504148;11135002）;中央高校基本科研业务费专项资金资助项目（lzujbky-2015-269）
中图分类号: O56

Coherent control of population transfer of the excited double states based on pulse shaping

1.
School of Nuclear Science and Technology, Lanzhou University, Lanzhou 730000, China

Corresponding author: LIU Zuoye, zyl@lzu.edu.cn

CLC number: O56

摘要: 为了实现红外飞秒脉冲的整形及调控，采用4f系统相位控制技术，实验搭建了脉冲整形装置，并利用整形脉冲对铷原子体系中激发双重态间的相干布居转移进行操控。结果表明，控制抽运脉冲的附加相位，可实现双重态中上激发态的饱和布居，通过修改附加相位函数可将上、下激发态的布居数反转。整形脉冲同样适用于其它的原子和分子系统的相干布居转移的操控。
- 激光物理 /
- 激发双重态 /
- 整形脉冲 /
- 相干布居转移
Abstract: In order to achieve the shaping and control of infrared femtosecond pulse, 4f system phase control technology was used and pulse shaping device was set up by experiment. By using pulse shaping, coherent of population transfer of the excited double states in the rubidium atoms system was controlled. The results show that saturation population can be realized in excited double state by controlling the additional phase of pumping pulse. Population of the upper and lower excited state can be reversed by modifying the function of additional phase. Coherent control of population transfer by pulse shaping can also be applied in other atom and molecular systems.
- laser physics /
- the excited double states /
- pulse shaping /
- coherent control of population transfer

[1]	DRNER R, MERGEL V, JAGUTZKI O,et al. Cold target recoil ion momentum spectroscopy:a momentum microscope to view atomic collision dynamics[J].Physics Reports, 2000, 330(2/3):95-192.
[2]	ULLRICH J, MOSHAMMER R, DORN A, et al. Recoil-ion and electron momentum spectroscopy:reaction-microscopes[J]. Reports on Progress in Physics, 2003, 66(9):1463-1545.
[3]	FANO U, COOPER J W. Spectral distribution of atomic oscillator strengths[J]. Reviews of Modern Physics, 1968, 40(3):441-507.
[4]	MATHIES R A, CRUZ C H B, POLLARD W T, et al. Direct observation of the femtosecond excited-state cis-trans isomerization in bacteriorhodopsin[J]. Science, 1988, 240(4853):777-779.
[5]	GOULIELMAKIS E, LOH Z H, WIRTH A, et al. Real-time observation of valence electron motion[J]. Nature, 2010, 466(7307):739-U7.
[6]	NICOLE C, BOUCHENE M A, ZAMITH S, et al.Saturation of wave-packet interferences:direct observation of spin precession in potassium atoms[J]. Physical Review, 1999,A60(3):R1755-R1758.
[7]	SOKELL E, ZAMITH S, BOUCHENE M A,et al. Polarization-dependent pump-probe studies in atomic fine-structure levels:towards the production of spin-polarized electrons[J]. Journal of Physics,2000, B33(11):2005-2015.
[8]	ZAMITH S, BOUCHENE M, SOKELL E,et al. Pump probe experiment in atomic fine structure levels:observation of the oscillation of an angular wavepacket[J]. European Physical Journal, 2000,D12(2):255-261.
[9]	BOUCHENE M A, ZAMITH S, GIRARD B. Spin-polarized electrons produced by a sequence of two femtosecond pulses. Calculation of differential and global polarization rates[J]. Journal of Physics, 2001, B34(8):1497-1512.
[10]	CHATEL B, BIGOURD D, WEBER S, et al.Coherent control of spin-orbit precession with shaped laser pulses[J]. Journal of Physics, 2008, B41(7):074023.
[11]	KATSUKI H, CHIBA H, MEIER C, et al.Actively Tailored spatiotemporal images of quantum interference on the picometer and femtosecond scales[J]. Physical Review Letters, 2009, 102(10):103602.
[12]	KATSUKI H, CHIBA H, GIRARD B,et al.Visualizing picometric quantum ripples of ultrafast wave-packet interference[J]. Science, 2006, 311(5767):1589-1592.
[13]	GOSWAMI D. Optical pulse shaping approaches to coherent control[J]. Physics Reports-Review Section of Physics Letters, 2003, 374(6):385-481.
[14]	BRIF C, CHAKRABARTI R, RABITZ H. Control of quantum phenomena:past, present and future[J]. New Journal of Physics, 2009, 12(2):2181-2188.
[15]	BARMES I, WITTE S, EIKEMA K S E.High-precision spectroscopy with counterpropagating femtosecond pulses[J]. Physical Review Letters, 2013,111(2):023007.
[16]	LEE S, LEE H G, CHO J, et al. Coherent control of multiphoton-ionization passage of excited-state rubidium atoms[J]. Physical Review, 2012,A86(4):045402.
[17]	HILDNER R, BRINKS D, van HULST N F.Femtosecond coherence and quantum control of single molecules at room temperature[J]. Nature Physics, 2011, 7(2):172-177.
[18]	LIU Z, OTT C, CAVALETTO S M,et al.Generation of high-frequency combs locked to atomic resonances by quantum phase modulation[J]. New Journal of Physics, 2014, 16(9):093005.
[19]	PRKELT A, WOLLENHAUPT M, ASSION A, et al. Compact, robust, and flexible setup for femtosecond pulse shaping[J]. Review of Scientific Instruments, 2003, 74(11):4950-4953.
[20]	LIU Z Y.Dynamic of multi-filament interaction and quantum phase control in atomic and molecular sytems[D]. Lanzhou:Lanzhou University, 2014:23-26(in Chinese).
[21]	NETZ R, FEURER T, ROBERTS G, et al.Coherent population dynamics of a three-level atom in spacetime[J]. Physical Review, 2002,A65(4):043406.
[22]	LIU Z Y, CAVALETTO S M, OTT C, et al. Phase reconstruction of strong-field excited systems by transient-absorption spectroscopy[J]. Physical Review Letters, 2015, 115(3):033003.

[1]	占剑 , 杨明江 . 脉冲YAG激光诱导放电击穿电压研究. 激光技术, 2009, 33(2): 138-140.
[2]	杨明惠 , 金琪 , 刘劲松 , 王可嘉 , 杨振刚 . 飞秒激光结合啁啾太赫兹脉冲控制CO分子取向. 激光技术, 2015, 39(6): 735-740. doi: 10.7510/jgjs.issn.1001-3806.2015.06.001
[3]	栗兴良 , 牛春晖 , 马牧燕 , 吕勇 . 单脉冲激光损伤CCD探测器的有限元仿真. 激光技术, 2016, 40(5): 730-733. doi: 10.7510/jgjs.issn.1001-3806.2016.05.023
[4]	赵洋 , 金光勇 , 李明欣 , 张巍 , 王頔 . 毫秒脉冲激光损伤CCD探测器的实验研究. 激光技术, 2017, 41(5): 632-636. doi: 10.7510/jgjs.issn.1001-3806.2017.05.003
[5]	孙秦 , 田雷超 , 武耀星 , 尹培琪 , 王均武 , 王新兵 , 左都罗 . 朗缪尔探针诊断脉冲激光锡等离子体特性. 激光技术, 2021, 45(1): 109-114. doi: 10.7510/jgjs.issn.1001-3806.2021.01.019
[6]	熊晗 , 刘三秋 , 廖晶晶 , 刘笑兰 . 短脉冲强激光在次临界密度等离子体中的传播. 激光技术, 2010, 34(2): 272-274,284. doi: 10.3969/j.issn.1001-3806.2010.02.035
[7]	黎小鹿 , 李俊 , 陶向阳 . 超短脉冲激光烧蚀半导体表面的热效应分析. 激光技术, 2007, 31(6): 624-626,629.
[8]	艾尔肯·扎克尔 , 阿不都热苏力·阿不都热西提 , 艾米尔丁·艾米都拉 . 不同激光脉冲驱动的尾场中正电子加速的研究. 激光技术, 2011, 35(6): 854-856. doi: 10.3969/j.issn.1001-3806.2011.06.034
[9]	杨燕飞 , 李廷帅 . 纳秒激光耦合金属靶辐射电磁脉冲的实验研究. 激光技术, 2020, 44(5): 647-651. doi: 10.7510/jgjs.issn.1001-3806.2020.05.021
[10]	赵刚 , 陈建国 , 张菁 , 黄强 . 飞秒光脉冲破坏阈值的解析分析. 激光技术, 2006, 30(1): 90-92.
[11]	黄艳 . 高斯-谢尔脉冲在单模光纤中的传输特性研究. 激光技术, 2019, 43(6): 841-845. doi: 10.7510/jgjs.issn.1001-3806.2019.06.020
[12]	饶连周 . J₀相关径向偏振涡旋光束紧聚焦的空间相干特性. 激光技术, 2021, 45(2): 240-245. doi: 10.7510/jgjs.issn.1001-3806.2021.02.020
[13]	赵廷靖 . 光阑对部分相干光束轴向偏振特性的影响. 激光技术, 2008, 32(4): 424-426,433.
[14]	唐芳 , 牛燕雄 , 张雏 , 陈燕 , 姜楠 , 杨海林 . 激光辐照皮肤组织的热效应解析计算研究. 激光技术, 2008, 32(5): 542-544.
[15]	史彭 , 辛宇 , 李隆 , 陈文 , 白冰 . 矩形截面Nd:GGG热容激光器热分析. 激光技术, 2011, 35(3): 305-307,333. doi: 10.3969/j.issn.1001-3806.2011.03.005
[16]	王纪俊 , 沈中华 , 倪晓武 , 许伯强 , 关建飞 , 陆建 . 透明薄膜/基底系统激光超声波的有限元数值研究. 激光技术, 2006, 30(2): 177-180.
[17]	邹晶 , 赵圣之 , 杨克建 , 李桂秋 . CCD测量LD端面抽运Nd：GdVO4固体激光器热焦距. 激光技术, 2006, 30(4): 422-424,428.
[18]	赵艳 , 沈中华 , 陆健 , 倪晓武 . 圆柱型涂层/基底系统中的激光超声表面波. 激光技术, 2006, 30(6): 647-649,666.
[19]	陈子琪 , 王新兵 , 左都罗 . CO2激光诱导液滴射流等离子体的实验研究. 激光技术, 2016, 40(6): 888-891. doi: 10.7510/jgjs.issn.1001-3806.2016.06.023
[20]	叶庆 . 偏置信号和噪声对单模激光随机共振的影响. 激光技术, 2017, 41(4): 602-605. doi: 10.7510/jgjs.issn.1001-3806.2017.04.029

点击查看大图

计量

文章访问数: 4385
HTML全文浏览量: 1932
PDF下载量: 319
被引次数: 0

姓名
邮箱
手机号码
标题
留言内容
验证码

留言板

基于脉冲整形的激发双重态间的相干布局操控

作者简介: 王贞浩(1994-),男,硕士研究生,现主要从事基于飞秒脉冲的瞬态吸收谱测量的研究。.

通讯作者: 刘作业, zyl@lzu.edu.cn

Coherent control of population transfer of the excited double states based on pulse shaping

Corresponding author: LIU Zuoye, zyl@lzu.edu.cn

计量

基于脉冲整形的激发双重态间的相干布局操控

通讯作者: 刘作业, zyl@lzu.edu.cn

作者简介: 王贞浩(1994-),男,硕士研究生,现主要从事基于飞秒脉冲的瞬态吸收谱测量的研究。

English Abstract

Coherent control of population transfer of the excited double states based on pulse shaping

Corresponding author: LIU Zuoye, zyl@lzu.edu.cn

全文HTML

目录

留言板

基于脉冲整形的激发双重态间的相干布局操控

作者简介: 王贞浩(1994-),男,硕士研究生,现主要从事基于飞秒脉冲的瞬态吸收谱测量的研究。.

通讯作者: 刘作业, zyl@lzu.edu.cn

Coherent control of population transfer of the excited double states based on pulse shaping

Corresponding author: LIU Zuoye, zyl@lzu.edu.cn

计量

出版历程

基于脉冲整形的激发双重态间的相干布局操控

通讯作者: 刘作业, zyl@lzu.edu.cn

作者简介: 王贞浩(1994-),男,硕士研究生,现主要从事基于飞秒脉冲的瞬态吸收谱测量的研究。

English Abstract

Coherent control of population transfer of the excited double states based on pulse shaping

Corresponding author: LIU Zuoye, zyl@lzu.edu.cn

全文HTML

目录